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A quantitative study on the degradation of whale bone lipids: implications for the preservation of fatty acids in marine sediments
Swedish Museum of Natural History, Department of Paleobiology.
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2015 (English)In: Organic Geochemistry, ISSN 0146-6380, E-ISSN 1873-5290, Vol. 89-90, p. 23-30Article in journal (Refereed) Published
Abstract [en]

The degradation and preservation affecting the biomarker record of ancient metazoa are not fully 33understood. We report on a five month experiment on the fate of fatty acids (FAs) during the degradation 34of recent whale vertebrae (Phocoena phocoena). Whale bones were analysed for extractable FAs and 35macromolecularly bound n-acyl compounds. Fresh bone showed extractable FAs dominated by 3616:1x7c, 16:0, 18:1x9c and 18:0. Calculated degradation rate constant (k) values showed a rapid 37decrease in FA concentration, with k values higher for unsaturated than for saturated compounds 38(e.g. 0.08/day for 18:1x9c, 0.05/day for 16:0). The appearance or increased abundance of distinctive 39methyl branched (e.g. i/ai-15:0 and -17:0, 10Me-16:0) and hydroxy FAs (e.g. 10OH-16:0 and 10OH- 4018:0) were observed, providing clear evidence for the microbial degradation of bone organic matter 41and an input of lipids from specialised bacteria. Catalytic hydropyrolysis (HyPy) of demineralised extrac- 42tion residues released up to 0.13% of the total n-C16 and n-C18 moieties in the degraded bones. This 43revealed that only a small, yet sizeable portion of bone-derived fatty acyl units was sequestered into 44(proto)kerogen during the earliest stages of degradation.

Place, publisher, year, edition, pages
2015. Vol. 89-90, p. 23-30
National Category
Geochemistry
Research subject
Ecosystems and species history
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URN: urn:nbn:se:nrm:diva-1437DOI: 10.1016/j.orggeochem.2015.09.005OAI: oai:DiVA.org:nrm-1437DiVA, id: diva2:875460
Available from: 2015-12-01 Created: 2015-12-01 Last updated: 2017-12-01Bibliographically approved

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